Abstract
The magnetic phase diagram and low-energy magnon excitations of structurally and magnetically chiral are reported. The specific heat and the static magnetization are investigated in magnetic fields up to 9 and 30 T, respectively, while the dynamic magnetic properties are probed by X-band as well as tunable high-frequency electron spin-resonance spectroscopy. Below K, we observe antiferromagnetic resonance modes which imply small but finite planar anisotropy showing up in a zero-field splitting of 20 GHz. The data are well described by means of an easy-plane two-sublattice model with the anisotropy field T. The exchange field T is obtained from the saturation field derived from the pulsed-field magnetization. A crucial role of the small anisotropy for the spin structure is reflected by competing antiferromagnetic phases appearing, at K, in small magnetic fields at T and T. We discuss the results in terms of spin reorientation and of small magnetic fields favoring helical spin structure over the cycloidal ground state which, at , is stabilized by the planar anisotropy. Above , short-range magnetic correlations up to K and magnetic entropy changes well above reflect the frustrated triangular arrangement of ions in .
2 More- Received 6 June 2016
- Revised 9 August 2016
DOI:https://doi.org/10.1103/PhysRevB.94.104408
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