Magnetic anisotropy and the phase diagram of chiral MnSb2O6

J. Werner, C. Koo, R. Klingeler, A. N. Vasiliev, Y. A. Ovchenkov, A. S. Polovkova, G. V. Raganyan, and E. A. Zvereva
Phys. Rev. B 94, 104408 – Published 6 September 2016

Abstract

The magnetic phase diagram and low-energy magnon excitations of structurally and magnetically chiral MnSb2O6 are reported. The specific heat and the static magnetization are investigated in magnetic fields up to 9 and 30 T, respectively, while the dynamic magnetic properties are probed by X-band as well as tunable high-frequency electron spin-resonance spectroscopy. Below TN=11.5 K, we observe antiferromagnetic resonance modes which imply small but finite planar anisotropy showing up in a zero-field splitting of 20 GHz. The data are well described by means of an easy-plane two-sublattice model with the anisotropy field BA=0.02 T. The exchange field BE=13 T is obtained from the saturation field derived from the pulsed-field magnetization. A crucial role of the small anisotropy for the spin structure is reflected by competing antiferromagnetic phases appearing, at T=2 K, in small magnetic fields at BC1 0.5 T and BC2=0.9 T. We discuss the results in terms of spin reorientation and of small magnetic fields favoring helical spin structure over the cycloidal ground state which, at B=0, is stabilized by the planar anisotropy. Above TN, short-range magnetic correlations up to 60 K and magnetic entropy changes well above TN reflect the frustrated triangular arrangement of Mn2+ ions in MnSb2O6.

  • Figure
  • Figure
  • Figure
  • Figure
  • Figure
  • Figure
  • Figure
2 More
  • Received 6 June 2016
  • Revised 9 August 2016

DOI:https://doi.org/10.1103/PhysRevB.94.104408

©2016 American Physical Society

Physics Subject Headings (PhySH)

Condensed Matter, Materials & Applied Physics

Authors & Affiliations

J. Werner, C. Koo, and R. Klingeler*

  • Kirchhoff Institute of Physics, Heidelberg University, INF 227, D-69120 Heidelberg, Germany and Centre for Advanced Materials, Heidelberg University, INF 225, 69120 Heidelberg, Germany

A. N. Vasiliev

  • Physics Faculty, M.V. Lomonosov Moscow State University, Moscow 119991, Russia; Theoretical Physics and Applied Mathematics Department, Ural Federal University, 620002 Ekaterinburg, Russia; and National University of Science and Technology “MISiS”, Moscow 119049, Russia

Y. A. Ovchenkov, A. S. Polovkova, G. V. Raganyan, and E. A. Zvereva

  • Physics Faculty, M.V. Lomonosov Moscow State University, Moscow 119991, Russia

  • *klingeler@kip.uni-hd.de

Article Text (Subscription Required)

Click to Expand

References (Subscription Required)

Click to Expand
Issue

Vol. 94, Iss. 10 — 1 September 2016

Reuse & Permissions
Access Options
Author publication services for translation and copyediting assistance advertisement

Authorization Required


×
×

Images

×

Sign up to receive regular email alerts from Physical Review B

Log In

Cancel
×

Search


Article Lookup

Paste a citation or DOI

Enter a citation
×