Abstract
Working on the transition of in , we provide the first detailed characterization of excitation-induced shifts in optical transition frequencies and demonstrate their exaggeration of nominally homogeneous dephasing rates. The shifts (found to vary in rough proportion to the number of ions excited and to be as small as one part in ) were identified through their unique signature in specially designed photon-echo experiments. The effects reported may constitute a rather general complication in optical measurements of homogeneous relaxation rates in solids.
- Received 3 January 1989
DOI:https://doi.org/10.1103/PhysRevLett.63.78
©1989 American Physical Society