Abstract
We report the first observation of photon antibunching in the photoluminescence from single carbon nanotubes. The emergence of a fast luminescence decay component under strong optical excitation indicates that Auger processes are partially responsible for inhibiting two-photon generation. Additionally, the presence of exciton localization at low temperatures ensures that nanotubes emit photons predominantly one by one. The fact that multiphoton emission probability can be smaller than 5% suggests that carbon nanotubes could be used as a source of single photons for applications in quantum cryptography.
- Received 3 December 2007
DOI:https://doi.org/10.1103/PhysRevLett.100.217401
©2008 American Physical Society
Synopsis
Single photon emission in the next dimension
Published 14 July 2008
Single photon emission is normally only observed in systems, such as atoms, that are quantum confined in all directions. Now, scientists have shown that carbon nanotubes, which are quasi-one-dimensional materials, can also act as single photon emitters.
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