Abstract
The thermal conductivity of single crystals was measured. Information on the inelastic scattering of electrons by various mechanisms for heat current was obtained, i.e., scattering by crystal-field splitting, level splitting accompanied with antiferromagnetic ordering, magnons, and short-range ordering. In Pr, Nd, and Ce, in the paramagnetic region, a pronounced decrease of the Lorentz number was observed below ∼20, ∼15, and ∼25 K, respectively, which indicates an increase of the inelastic scattering. By comparing the temperature dependence on the spin-lattice relaxation rate in the first two compounds, it is found to be due to short-range magnetic ordering in these compounds. In Ce, a decrease of below ∼25 K should be due to short-range quadrupole ordering, which may be related to the unusual behavior of and the unusual properties in the paramagnetic region in this compound. of Sm shows a pronounced increase below ∼40 K, that is related to the gap opening in this compound.
- Received 1 May 1996
DOI:https://doi.org/10.1103/PhysRevB.54.R5207
©1996 American Physical Society