Abstract
Raman spectra of (spin S=1) reveal an anomalously broad two-magnon feature whose relative width is comparable to that shown by (S=1/2) and other antiferromagnetic copper oxides. The magnetic continuum is strongly coupled to a nearby phonon, whose scattering amplitude interferes with it. These results question the view that the width enhancement in the cuprates stems from large quantum fluctuations intrinsic to S=1/2 systems. It is proposed that the anomaly is due instead to magnon decay involving strong magnetostrictive coupling to phonons.
- Received 16 December 1993
DOI:https://doi.org/10.1103/PhysRevB.49.4352
©1994 American Physical Society