Geometrical Frustration in the Ferromagnetic Pyrochlore Ho2Ti2O7

M. J. Harris, S. T. Bramwell, D. F. McMorrow, T. Zeiske, and K. W. Godfrey
Phys. Rev. Lett. 79, 2554 – Published 29 September 1997
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Abstract

We report a detailed study of the pyrochlore Ho2Ti2O7, in which the magnetic ions (Ho3+) are ferromagnetically coupled with J1K. We show that the presence of local Ising anisotropy leads to a geometrically frustrated ground state, preventing long-range magnetic order down to at least 0.05 K. However, unlike in the case of a frustrated antiferromagnet, this disorder is principally static. In a magnetic field, the ground-state degeneracy is broken and ordered magnetic phases are formed which display an unusual history dependence due to the slow dynamics of the system. These results represent the first experimental evidence for geometrical frustration in a ferromagnetic system.

  • Received 19 May 1997

DOI:https://doi.org/10.1103/PhysRevLett.79.2554

©1997 American Physical Society

Authors & Affiliations

M. J. Harris1, S. T. Bramwell2, D. F. McMorrow3, T. Zeiske4, and K. W. Godfrey5

  • 1ISIS Facility, Rutherford Appleton Laboratory, Chilton, Didcot, Oxon, OX11 0QX, United Kingdom
  • 2Department of Chemistry, University College London, 20 Gordon Street, London, WC1H 0AJ, United Kingdom
  • 3Department of Solid State Physics, Risø National Laboratory, DK-4000 Roskilde, Denmark
  • 4Institut für Kristallographie, Universität Tübingen, c.o. Hahn-Meitner-Institut, Glienickerstrasse 100, D-14109, Berlin, Germany
  • 5Oxford Physics, Clarendon Laboratory, Parks Road, Oxford, OX1 3PU, United Kingdom

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Vol. 79, Iss. 13 — 29 September 1997

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