Abstract
The magnetic susceptibility of single-crystal , a linear (spin-1/2) chain compound, was measured. The susceptibilities in all the directions rapidly drop to small constant values with decreasing temperature below a phase transition temperature near 14 K. The magnetic-field dependence of the transition temperature quantitatively agrees with both theoretical predictions and experimental results for organic spin-Peierls systems. This Letter is the first report of an unambiguous determination of the existence of the spin-Peierls transition in an inorganic compound.
- Received 4 January 1993
DOI:https://doi.org/10.1103/PhysRevLett.70.3651
©1993 American Physical Society