Simple Theory for the Dynamics of Mean-Field-Like Models of Glass-Forming Fluids

Grzegorz Szamel
Phys. Rev. Lett. 119, 155502 – Published 13 October 2017
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Abstract

We propose a simple theory for the dynamics of model glass-forming fluids, which should be solvable using a mean-field-like approach. The theory is based on transparent physical assumptions, which can be tested in computer simulations. The theory predicts an ergodicity-breaking transition that is identical to the so-called dynamic transition predicted within the replica approach. Thus, it can provide the missing dynamic component of the random first order transition framework. In the large-dimensional limit the theory reproduces the result of a recent exact calculation of Maimbourg et al. [Phys. Rev. Lett. 116, 015902 (2016)]. Our approach provides an alternative, physically motivated derivation of this result.

  • Received 9 May 2017

DOI:https://doi.org/10.1103/PhysRevLett.119.155502

© 2017 American Physical Society

Physics Subject Headings (PhySH)

Condensed Matter, Materials & Applied PhysicsStatistical Physics & Thermodynamics

Authors & Affiliations

Grzegorz Szamel

  • Department of Chemistry, Colorado State University, Fort Collins, Colorado 80523, USA

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Issue

Vol. 119, Iss. 15 — 13 October 2017

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