Abstract
We investigate the temporal evolution of molecular frame angular distributions of Auger electrons emitted during ultrafast dissociation of HCl following a resonant single-photon excitation. The electron emission pattern changes its shape from that of a molecular orbital to that of an atomic state as the system evolves from a molecule into two separated atoms.
- Received 27 September 2016
DOI:https://doi.org/10.1103/PhysRevLett.117.243002
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