Strong paramagnon scattering in single atom Pd contacts

V. Schendel, C. Barreteau, M. Brandbyge, B. Borca, I. Pentegov, U. Schlickum, M. Ternes, P. Wahl, and K. Kern
Phys. Rev. B 96, 035155 – Published 31 July 2017

Abstract

Among all transition metals, palladium (Pd) has the highest density of states at the Fermi energy at low temperatures yet does not fulfill the Stoner criterion for ferromagnetism. However, close proximity to magnetism renders it a nearly ferromagnetic metal, which hosts paramagnons, strongly damped spin fluctuations. Here we compare the total and the differential conductance of monoatomic contacts consisting of single Pd and cobalt (Co) atoms between Pd electrodes. Transport measurements reveal a conductance for Co of 1G0, while for Pd we obtain 2G0. The differential conductance of monoatomic Pd contacts shows a reduction with increasing bias, which gives rise to a peculiar Λ-shaped spectrum. Supported by theoretical calculations, we correlate this finding with the lifetime of hot quasiparticles in Pd, which is strongly influenced by paramagnon scattering. In contrast to this, Co adatoms locally induce magnetic order, and transport through single cobalt atoms remains unaffected by paramagnon scattering, consistent with theory.

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  • Received 8 February 2017

DOI:https://doi.org/10.1103/PhysRevB.96.035155

©2017 American Physical Society

Physics Subject Headings (PhySH)

Condensed Matter, Materials & Applied Physics

Authors & Affiliations

V. Schendel1,*, C. Barreteau2,3, M. Brandbyge3, B. Borca1, I. Pentegov1, U. Schlickum1, M. Ternes1, P. Wahl4,1, and K. Kern1,5

  • 1Max-Planck-Institut für Festkörperforschung, Heisenbergstraße 1, 70569 Stuttgart, Germany
  • 2Service de Physique de L'Etat Condensé (SPEC), CEA, CNRS, Université Paris-Saclay, CEA Saclay, 91191 Gif-sur-Yvette Cedex, France
  • 3Department of Micro- and Nanotechnology, Technical University of Denmark, Ørsteds Plads, Building 345B, DK-2800 Kongens Lyngby, Denmark
  • 4SUPA, School of Physics and Astronomy, University of St. Andrews, Scotland, United Kingdom
  • 5Institut de Physique, Ecole Polytechnique Fédérale de Lausanne, 1015 Lausanne, Switzerland

  • *Corresponding author: verena.schendel@kit.edu

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Issue

Vol. 96, Iss. 3 — 15 July 2017

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