Abstract
Examples of materials where an “order by disorder” mechanism is at play to select a particular ground state are scarce. It has recently been proposed, however, that the antiferromagnetic XY pyrochlore reveals a most convincing case of this mechanism, with the observation of a spin gap at zone centers having recently been interpreted as a corroboration of this physics. Here we argue, however, that the anisotropy generated by the interaction-induced admixing between the crystal-field ground and excited levels provides for an alternative mechanism. It especially predicts the opening of a spin gap of about 15 , which is of the same order of magnitude as the one observed experimentally. We report high-resolution inelastic neutron scattering data which can be well understood within this scenario.
- Received 28 June 2014
- Revised 31 July 2014
DOI:https://doi.org/10.1103/PhysRevB.90.060410
©2014 American Physical Society