Photon-assisted tunneling through molecular conduction junctions with graphene electrodes

Boris D. Fainberg
Phys. Rev. B 88, 245435 – Published 23 December 2013

Abstract

Graphene electrodes provide a suitable alternative to metal contacts in molecular conduction nanojunctions. Here, we propose to use graphene electrodes as a platform for effective photon assisted tunneling through molecular conduction nanojunctions. We predict dramatic increasing currents evaluated at side-band energies nω (n is a whole number) related to the modification of graphene gapless spectrum under the action of external electromagnetic field of frequency ω. A side benefit of using doped graphene electrodes is the polarization control of photocurrent related to the processes occurring either in the graphene electrodes or in the molecular bridge. The latter processes are accompanied by surface plasmon excitation in the graphene sheet that makes them more efficient. Our results illustrate the potential of graphene contacts in coherent control of photocurrent in molecular electronics, supporting the possibility of single-molecule devices.

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  • Received 12 September 2013
  • Revised 29 October 2013

DOI:https://doi.org/10.1103/PhysRevB.88.245435

©2013 American Physical Society

Authors & Affiliations

Boris D. Fainberg*

  • Faculty of Science, Holon Institute of Technology, 5810201 Holon, Israel
  • and School of Chemistry, Tel-Aviv University, 69978 Tel-Aviv, Israel

  • *fainberg@hit.ac.il

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Issue

Vol. 88, Iss. 24 — 15 December 2013

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