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Ground-state order and spin-lattice coupling in tetrahedral spin systems Cu2Te2O5X2 (X=Br or Cl)

M. Prester, A. Smontara, I. Živković, A. Bilušić, D. Drobac, H. Berger, and F. Bussy
Phys. Rev. B 69, 180401(R) – Published 10 May 2004
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Abstract

High-resolution ac susceptibility and thermal conductivity measurement on Cu2Te2O5X2(X=Br,Cl) single crystals are reported. For Br-sample, sample dependence prevents one from distinguishing between possibilities of magnetically ordered and spin-singlet ground states. In Cl-sample a three-dimensional transition at 18.5 K is accompanied by almost isotropic behavior of susceptibility and almost switching behavior of thermal conductivity. Thermal conductivity studies suggest the presence of a tremendous spin-lattice coupling characterizing Cl- but not Br-sample. Below the transition Cl-sample is in a complex magnetic state involving AF order but also the elements consistent with the presence of a gap in the excitation spectrum.

  • Received 10 December 2003

DOI:https://doi.org/10.1103/PhysRevB.69.180401

©2004 American Physical Society

Authors & Affiliations

M. Prester1,*, A. Smontara1,†, I. Živković1, A. Bilušić1, D. Drobac1, H. Berger2, and F. Bussy3

  • 1Institute of Physics, P.O. Box 304, HR-10 000, Zagreb, Croatia
  • 2Institut de Physique de la Matière Complexe, EPFL, CH-1015 Lausanne, Switzerland
  • 3Institute of Mineralogy and Geochemistry BFSH-2, University of Lausanne, CH-1015 Lausanne, Switzerland

  • *Electronic address: prester@ifs.hr
  • Electronic address: ana@ifs.hr

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Vol. 69, Iss. 18 — 1 May 2004

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