Pseudogapped Fermi surfaces of 1TTaS2 and 1TTaSe2: A charge density wave effect

M. Bovet, D. Popović, F. Clerc, C. Koitzsch, U. Probst, E. Bucher, H. Berger, D. Naumović, and P. Aebi
Phys. Rev. B 69, 125117 – Published 30 March 2004
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Abstract

We report room temperature angle-resolved photoemission experiments on 1TTaS2 and 1TTaSe2 complemented by density-functional theory calculations. Fermi-surface mapping experiments in the charge-density wave (CDW) phase are similar for the two compounds and do not show symmetries due to the CDW-induced new Brillouin zones. However, the band structure a few eV below the Fermi level (EF) displays a clear modulation that we relate, in both cases, to the CDW. At EF, the spectral weight distribution reflects the band structure of the normal state, but no clear quasiparticle crossing is located. Near the zone center Γ¯, CDW-split quasilocalized Ta dz2 subbands are observed in the vicinity of EF. For 1TTaS2 and 1TTaSe2, they are thermally populated slightly above EF and close to EF, respectively. The observed behavior can be understood in terms of the CDW reconstructed, spectral function weighted band structure.

  • Received 26 September 2003

DOI:https://doi.org/10.1103/PhysRevB.69.125117

©2004 American Physical Society

Authors & Affiliations

M. Bovet1, D. Popović2, F. Clerc3, C. Koitzsch3, U. Probst4, E. Bucher4, H. Berger5, D. Naumović1, and P. Aebi3

  • 1Département de Physique, Université de Fribourg, Pérolles, CH-1700 Fribourg, Switzerland
  • 2Experimentalphysik, Universität des Saarlandes, D-66123 Saarbrücken, Germany
  • 3Institut de Physique, Université de Neuchâtel, CH-2000 Neuchâtel, Switzerland
  • 4Fachbereich Physik, Universität Konstanz, D-78457 Konstanz, Germany
  • 5Institut de Physique Appliquée, EPFL, CH-1015 Lausanne, Switzerland

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Vol. 69, Iss. 12 — 15 March 2004

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