Abstract
We report room temperature angle-resolved photoemission experiments on and complemented by density-functional theory calculations. Fermi-surface mapping experiments in the charge-density wave (CDW) phase are similar for the two compounds and do not show symmetries due to the CDW-induced new Brillouin zones. However, the band structure a few eV below the Fermi level displays a clear modulation that we relate, in both cases, to the CDW. At the spectral weight distribution reflects the band structure of the normal state, but no clear quasiparticle crossing is located. Near the zone center CDW-split quasilocalized Ta subbands are observed in the vicinity of For and they are thermally populated slightly above and close to respectively. The observed behavior can be understood in terms of the CDW reconstructed, spectral function weighted band structure.
- Received 26 September 2003
DOI:https://doi.org/10.1103/PhysRevB.69.125117
©2004 American Physical Society