Abstract
is a rare example of a nearly two-dimensional Heisenberg antiferromagnet on a triangular lattice. Magnetic resonance spectra and magnetization curves reveal that the system has a layered spin structure with six magnetic sublattices. The sublattices within a layer are arranged in a triangular manner with the magnetization vectors apart. The phase diagram, containing at least five different magnetic phases is constructed. In zero field, undergoes a phase transition at into a noncollinear triangular spin structure with all the spins confined in the basal plane. The application of an in-plane magnetic field induces a collinear spin state between the fields and and produces a magnetization plateau at one-third of the saturation moment. Both the ESR and the magnetization measurements also clearly indicate an additional first-order phase transition in a field of 35 kOe. The exact nature of this phase transition is uncertain.
- Received 10 October 2002
DOI:https://doi.org/10.1103/PhysRevB.67.094434
©2003 American Physical Society