Pump-probe spectroscopy using quantum light with two-photon coincidence detection

F. Schlawin, K. E. Dorfman, and S. Mukamel
Phys. Rev. A 93, 023807 – Published 3 February 2016

Abstract

We propose a pump-probe signal, whereby the sample is excited by a classical pulse, and—after a variable time delay—probed by a photon from an entangled pair, which is finally detected in coincidence with its twin. This setup offers an improved time and frequency resolution compared to a classical pump-probe signal, and can be used to enhance or suppress selected resonances.

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  • Received 9 September 2015
  • Revised 9 November 2015

DOI:https://doi.org/10.1103/PhysRevA.93.023807

©2016 American Physical Society

Physics Subject Headings (PhySH)

Atomic, Molecular & Optical

Authors & Affiliations

F. Schlawin1,*, K. E. Dorfman2, and S. Mukamel2

  • 1Physikalisches Institut, Albert-Ludwigs-Universität Freiburg, Hermann-Herder-Straße 3, 79104 Freiburg, Germany
  • 2Department of Chemistry, University of California, Irvine, California 92697, USA

  • *frank.schlawin@physik.uni-freiburg.de

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Issue

Vol. 93, Iss. 2 — February 2016

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