Forbidden nature of multipolar contributions to second-harmonic generation in isotropic fluids

David L. Andrews and Nick P. Blake
Phys. Rev. A 38, 3113 – Published 1 September 1988
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Abstract

Using a molecular theory of harmonic generation developed within the framework of quantum electrodynamics, we prove that second-harmonic generation is forbidden in isotropic fluids to all levels of multipolar approximation.

  • Received 16 May 1988

DOI:https://doi.org/10.1103/PhysRevA.38.3113

©1988 American Physical Society

Authors & Affiliations

David L. Andrews and Nick P. Blake

  • School of Chemical Sciences, University of East Anglia, Norwich NR4 7TJ, United Kingdom

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Issue

Vol. 38, Iss. 6 — September 1988

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