Phys. Rev. Lett. 92, 237401 (2004) [4 pages]

Imaging Density Disturbances in Water with a 41.3-Attosecond Time Resolution

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P. Abbamonte1 *, K. D. Finkelstein2, M. D. Collins1, and S. M. Gruner1,2
1Department of Physics, Cornell University, Ithaca, New York 14853-2501, USA
2Cornell High Energy Synchrotron Source, Cornell University, Ithaca, New York 14853-2501, USA

Featured in Phys. Rev. Focus Received 15 November 2003; published 11 June 2004

We show that the momentum flexibility of inelastic x-ray scattering may be exploited to invert its loss function, allowing real time imaging of density disturbances in a medium. We show the disturbance arising from a point source in liquid water, with a resolution of 41.3 attoseconds (4.13×10-17   s) and 1.27   Å (1.27×10-8   cm). This result is used to determine the structure of the electron cloud around a photoexcited chromophore in solution, as well as the wake generated in water by a 9 MeV gold ion. We draw an analogy with pump-probe techniques and suggest that energy-loss scattering may be applied more generally to the study of attosecond phenomena.


©2004 The American Physical Society

URL: http://link.aps.org/abstract/PRL/v92/e237401
DOI: 10.1103/PhysRevLett.92.237401
PACS: 78.70.Ck, 87.64.Gb

* Present address: Building 725D, Brookhaven National Laboratory, Upton, NY 11973, USA.

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