Anomaly of the Nonergodicity Parameter and Crossover to White Noise in the Fast Relaxation Spectrum of a Simple Glass Former

S. V. Adichtchev, St. Benkhof, Th. Blochowicz, V. N. Novikov, E. Rössler, Ch. Tschirwitz, and J. Wiedersich
Phys. Rev. Lett. 88, 055703 – Published 22 January 2002
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Abstract

We present quasielastic light scattering and dielectric spectra of the glass former α-picoline. At high temperatures the evolution of the susceptibility minimum is well described by the mode coupling theory (MCT). Below the critical temperature Tc the simple scaling laws of MCT fail due to the appearance of the excess wing of the α process, which shows a universal evolution as a function of log10τα. Taking this into account, however, we observe the predicted cusplike anomaly of the nonergodicity parameter as well as a crossover to “white noise.”

  • Received 20 August 2001

DOI:https://doi.org/10.1103/PhysRevLett.88.055703

©2002 American Physical Society

Authors & Affiliations

S. V. Adichtchev1, St. Benkhof1, Th. Blochowicz1, V. N. Novikov1, E. Rössler1,*, Ch. Tschirwitz1, and J. Wiedersich1,2

  • 1Physikalisches Institut EP II, Universität Bayreuth, 95440 Bayreuth, Germany
  • 2Technische Universität München, Lehrstuhl für Physik Weihenstephan, Vöttinger Strasse 40, 85350 Freising, Germany

  • *Corresponding author.

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Vol. 88, Iss. 5 — 4 February 2002

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