Abstract
O x-ray absorption study of the Mott insulator shows that the orbital population of the band dramatically changes with temperature. In addition, spin-resolved circularly polarized photoemission study of shows that a substantial orbital angular momentum is induced in the Ru band. Based on the experimental results and model Hartree-Fock calculations, we argue that the cooperation between the strong spin-orbit coupling in the Ru band and the small distortion of the octahedra causes the interesting changeover of the spin and orbital anisotropy as a function of temperature.
- Received 10 October 2000
DOI:https://doi.org/10.1103/PhysRevLett.87.077202
©2001 American Physical Society