Role of Unstable Directions in the Equilibrium and Aging Dynamics of Supercooled Liquids

Claudio Donati, Francesco Sciortino, and Piero Tartaglia
Phys. Rev. Lett. 85, 1464 – Published 14 August 2000
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Abstract

The connectivity of the potential energy landscape in supercooled atomic liquids is investigated through a calculation of the instantaneous normal modes spectrum and a detailed analysis of the unstable directions in configuration space. We confirm the hypothesis that the mode-coupling critical temperature is the T at which the dynamics crosses over from free to activated exploration of configuration space. We also observe changes in the local connectivity of configuration space sampled during aging, following a temperature jump from a liquid to a glassy state.

  • Received 22 December 1999

DOI:https://doi.org/10.1103/PhysRevLett.85.1464

©2000 American Physical Society

Authors & Affiliations

Claudio Donati, Francesco Sciortino, and Piero Tartaglia

  • Dipartimento di Fisica, Universita' di Roma “La Sapienza”, Istituto Nazionale per la Fisica della Materia, Piazzale Aldo Moro 2, I-00185, Roma, Italy

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Vol. 85, Iss. 7 — 14 August 2000

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