Abstract
Coherent acoustic phonons in PbS quantum dots are observed using femtosecond optical techniques. This is the first observation of coherent acoustic phonons in a semiconductor quantum dot; the phonons are generated through the deformation-potential coupling to the quantum-dot exciton. The acoustic modes are weakly damped, and we also find extremely weak coupling ( ) to the optical modes. These conclusions have important consequences for the vibronic nature of the exciton transition in the quantum dot and its dephasing.
- Received 10 July 1997
DOI:https://doi.org/10.1103/PhysRevLett.79.5102
©1997 American Physical Society