Photon antibunching in the fluorescence of a single dye molecule trapped in a solid

Th. Basché, W. E. Moerner, M. Orrit, and H. Talon
Phys. Rev. Lett. 69, 1516 – Published 7 September 1992
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Abstract

The correlation between fluorescence photons emitted by an optically pumped single molecule of pentacene in a p-terphenyl host has been investigated at short times. The correlation function shows photon antibunching, a unique feature of a nonclassical radiation field, which decreases if two molecules rather than one are pumped at the same time. The peculiarities of the correlation function for a three-level molecule are discussed and the theoretical description outlined.

  • Received 18 May 1992

DOI:https://doi.org/10.1103/PhysRevLett.69.1516

©1992 American Physical Society

Authors & Affiliations

Th. Basché and W. E. Moerner

  • IBM Research Division, Almaden Research Center, San Jose, California 95120

M. Orrit and H. Talon

  • Centre de Physique Moléculaire Optique et Hertzienne, CNRS Université de Bordeaux I, Talence, France

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Vol. 69, Iss. 10 — 7 September 1992

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