Softening of the H2+ molecular bond in intense laser fields

P. H. Bucksbaum, A. Zavriyev, H. G. Muller, and D. W. Schumacher
Phys. Rev. Lett. 64, 1883 – Published 16 April 1990
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Abstract

We report a new kind of multiphoton dissociation in intense laser fields. H2+ molecular ions were formed in above-threshold ionization of H2 gas by intense 532-nm, 100-ps laser pulses. Observations suggest that multiphoton couplings soften the molecular bond, resulting in dissociation at laser intensities over 50 TW/cm2. The ion-dissociation spectra have multiple peaks caused by multiphoton transitions during dissociation of H2+.

  • Received 26 October 1989

DOI:https://doi.org/10.1103/PhysRevLett.64.1883

©1990 American Physical Society

Authors & Affiliations

P. H. Bucksbaum, A. Zavriyev, H. G. Muller, and D. W. Schumacher

  • AT&T Bell Laboratories, Murray Hill, New Jersey 07974

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Issue

Vol. 64, Iss. 16 — 16 April 1990

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