Abstract
We report a new kind of multiphoton dissociation in intense laser fields. molecular ions were formed in above-threshold ionization of gas by intense 532-nm, 100-ps laser pulses. Observations suggest that multiphoton couplings soften the molecular bond, resulting in dissociation at laser intensities over 50 TW/. The ion-dissociation spectra have multiple peaks caused by multiphoton transitions during dissociation of .
- Received 26 October 1989
DOI:https://doi.org/10.1103/PhysRevLett.64.1883
©1990 American Physical Society