Abstract
Exciton decoherence (dephasing) properties are examined for the effects of biexcitons in quantum dots. The dephasing time of higher exciton states is measured from the linewidths of discrete exciton absorption lines by employing a high-energy-resolution microphotoluminescence excitation method in single isolated quantum dots. The excitation intensity dependence and temperature dependence of the exciton linewidth are used to consider the effects of exciton-biexciton and exciton-phonon interactions. The excitation intensity dependence reveals that the exciton-biexciton interaction contributes crucially to the exciton dephasing processes. A numerical calculation undertaken with a density-matrix method interprets this result as an enhancement of the power broadening effect due to coherent coupling between excitons and biexcitons. The temperature dependence indicates that the exciton-biexciton interaction dominates the exciton-phonon interaction below 40 K. These results provide a guideline for achieving a long-lived coherence in quantum dots, which is a key to the implementation of quantum information processing.
- Received 4 September 2003
- Accepted 4 September 2003
DOI:https://doi.org/10.1103/PhysRevB.69.155328
©2004 American Physical Society