Abstract
The complex magnetic transitions and superconductivity of were studied via the dependence of the heat capacity on temperature and in-plane field angle. We provide an extended, comprehensive magnetic phase diagram for and based on the thermodynamic measurements. Three magnetic transitions and the superconducting transition were clearly observed. The 5.2 K transition shows a hysteresis with temperature, indicating the first-order nature of the transition at The 6 K transition namely the onset of the long-range ordering, displays a dramatic in-plane anisotropy: increases with increasing magnetic field for while it decreases with increasing field for The anomalous anisotropy in indicates that the transition is related to the a-axis spiral structure. The 5.5 K transition shows similar behavior to the 5.2 K transition, i.e., a small in-plane anisotropy and scaling with Ising model. This last transition is ascribed to the change from dominant phase to dominant phase.
- Received 2 July 2003
DOI:https://doi.org/10.1103/PhysRevB.69.054505
©2004 American Physical Society