Tunneling broadening of vibrational sidebands in molecular transistors

Karsten Flensberg
Phys. Rev. B 68, 205323 – Published 24 November 2003
PDFExport Citation

Abstract

Transport through molecular quantum dots coupled to a single vibration mode is studied in the case with strong coupling to the leads. We use an expansion in the correlation between electrons on the molecule and electrons in the leads, and show that the tunneling broadening is strongly suppressed by the combination of the Pauli principle and the quantization of the oscillator. As a consequence the first Frank-Condon step is sharper than the higher order ones, and its width, when compared to the bare tunneling strength, is reduced by the overlap between the ground states of the displaced and nondisplaced oscillators.

  • Received 16 June 2003

DOI:https://doi.org/10.1103/PhysRevB.68.205323

©2003 American Physical Society

Authors & Affiliations

Karsten Flensberg

  • Laboratory of Atomic and Solid State Physics, Cornell University, Ithaca, NY 14853, USA
  • Ørsted Laboratory, Niels Bohr Institute fAPG, Universitetsparken 5, 2100 Copenhagen, Denmark

References (Subscription Required)

Click to Expand
Issue

Vol. 68, Iss. 20 — 15 November 2003

Reuse & Permissions
Access Options
Author publication services for translation and copyediting assistance advertisement

Authorization Required


×
×

Images

×

Sign up to receive regular email alerts from Physical Review B

Log In

Cancel
×

Search


Article Lookup

Paste a citation or DOI

Enter a citation
×