Low-temperature magnetic order and spin dynamics in YbRh2Si2

K. Ishida, D. E. MacLaughlin, Ben-Li Young, K. Okamoto, Y. Kawasaki, Y. Kitaoka, G. J. Nieuwenhuys, R. H. Heffner, O. O. Bernal, W. Higemoto, A. Koda, R. Kadono, O. Trovarelli, C. Geibel, and F. Steglich
Phys. Rev. B 68, 184401 – Published 3 November 2003
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Abstract

Muon spin rotation and relaxation experiments have been carried out in single crystals of YbRh2Si2, a compound that exhibits non-Fermi-liquid (NFL) behavior associated with a quantum critical point (QCP) at T=0. The zero-field muon relaxation rate is found to be independent of temperature down to 100 mK but to increase below 70mK, which suggests magnetic order at low temperatures. From the relation between the internal field at the μ+ stopping site and the hyperfine coupling constant the ordered Yb3+ moment is very small, 2×103μB. Muon spin rotation linewidths in a transverse field of 6 kOe indicate a homogeneous susceptibility down to 2 K, which is an order of magnitude lower than the characteristic (Kondo) temperature TK25K. This is evidence against the importance of disorder-driven NFL mechanisms in YbRh2Si2. In longitudinal magnetic fields the muon spin-lattice relaxation function G(t) is exponential, again indicative of a homogeneous system. The relaxation obeys the time-field scaling relation G(t,H)=G(t/H), which suggests long-lived spin correlations at low temperatures. The Yb3+ spin dynamics derived from muon spin relaxation appear to be intimately related to critical magnetic fluctuations near the QCP.

  • Received 19 March 2003

DOI:https://doi.org/10.1103/PhysRevB.68.184401

©2003 American Physical Society

Authors & Affiliations

K. Ishida1,2,*, D. E. MacLaughlin1, Ben-Li Young1, K. Okamoto2, Y. Kawasaki2,†, Y. Kitaoka2, G. J. Nieuwenhuys3, R. H. Heffner4, O. O. Bernal5, W. Higemoto6, A. Koda6, R. Kadono6, O. Trovarelli7, C. Geibel7, and F. Steglich7

  • 1Department of Physics, University of California, Riverside, California 92521-0413, USA
  • 2Department of Physical Science, Graduate School of Engineering Science, Osaka University, Toyonaka, Osaka 560-8531, Japan
  • 3Kamerlingh Onnes Laboratory, Leiden University, 2500 RA Leiden, The Netherlands
  • 4MS K764, Los Alamos National Laboratory, Los Alamos, New Mexico 87545, USA
  • 5Department of Physics and Astronomy, California State University, Los Angeles, California 90032, USA
  • 6Meson Science laboratory, Institute of Materials Structure Science, High Energy Accelerator Research Organization (KEK), 1-1 Oho, Tsukuba, Ibaraki 305-0801, Japan
  • 7Max-Planck Institute for Chemical Physics of Solids, D-01187 Dresden, Germany

  • *Present address: Department of Physics, Kyoto University, Kyoto 606-8502, Japan.
  • Present address: Department of Physics, Faculty of Engineering, Tokushima University, Tokushima 770-8506, Japan.

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Vol. 68, Iss. 18 — 1 November 2003

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