Magnetic state of Yb in Kondo-lattice YbNi2B2C

A. T. Boothroyd, J. P. Barratt, P. Bonville, P. C. Canfield, A. Murani, A. R. Wildes, and R. I. Bewley
Phys. Rev. B 67, 104407 – Published 14 March 2003
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Abstract

We report neutron-scattering experiments performed to investigate the dynamic magnetic properties of the Kondo-lattice compound YbNi2B2C. The spectrum of magnetic excitations is found to be broad, extending up to at least 150 meV, and contains inelastic peaks centered near 18 meV and 43 meV. At low energies, we observe quasielastic scattering with a width Γ=2.1 meV. The results suggest a Yb3+ ground state with predominantly localized 4f electrons subject to (i) a crystalline electric-field (CEF) potential, and (ii) a Kondo interaction, which at low temperatures is about an order of magnitude smaller than the CEF interaction. From an analysis of the dynamic magnetic response, we conclude that the crystalline electric field acting on the Yb ions has a similar anisotropy to that in other RNi2B2C compounds, but is uniformly enhanced by almost a factor of 2. The static and dynamic magnetic properties of YbNi2B2C are found to be reconciled quite well by means of an approximation scheme to the Anderson impurity model, and this procedure also indicates that the effective Kondo interaction varies with temperature due to the crystal-field splitting. We discuss the nature of the correlated-electron ground state of YbNi2B2C based on these and other experimental results, and suggest that this compound might be close to a quantum critical point on the nonmagnetic side.

  • Received 18 November 2002

DOI:https://doi.org/10.1103/PhysRevB.67.104407

©2003 American Physical Society

Authors & Affiliations

A. T. Boothroyd*

  • Department of Physics, Oxford University, Oxford OX1 3PU, United Kingdom

J. P. Barratt

  • Department of Physics, Oxford University, Oxford OX1 3PU, United Kingdom
  • Institut Laue-Langevin, Boîte Postale 156, 38042 Grenoble Cedex 9, France

P. Bonville

  • Centre d’Etudes de Saclay, DSM-DRECAM, Service de Physique de l’Etat Condensé, 91191 Gif-sur-Yvette Cedex, France

P. C. Canfield

  • Iowa State University and Ames Laboratory, Ames, Iowa 50011

A. Murani and A. R. Wildes

  • Institut Laue-Langevin, Boîte Postale 156, 38042 Grenoble Cedex 9, France

R. I. Bewley

  • ISIS Facility, Rutherford Appleton Laboratory, Chilton, Didcot OX11 0QX, United Kingdom

  • *Electronic address: a.boothroyd1@physics.ox.ac.uk; URL: http://xray.physics.ox.ac.uk/Boothroyd

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Issue

Vol. 67, Iss. 10 — 1 March 2003

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