Abstract
High-field electron-spin-resonance (ESR) experiments have been carried out in single crystals of in the concentration range Different quasioptical arrangements have been utilized for frequencies and for magnetic fields A splitting of the antiferromagnetic resonance (AFMR) mode is observed in the magnetic field for the parent compound in agreement with the antiferromagnetic structure of this material. Abrupt changes in the AFMR frequencies have been observed around and were attributed to a transition between a pure antiferromagnetic and a canted state. For increasing Sr doping the observed AFMR modes are split even in a zero field, which can be naturally explained using a concept of a canted magnetic structure for In the ESR spectra are consistent with the ferromagnetic and metallic state. The lines of ferromagnetic resonance and ferromagnetic antiresonance can be clearly observed. For intermediate concentrations complicated ESR spectra were observed, which can be well explained by a single ferromagnetic resonance mode and taking electrodynamic effects into account.
- Received 1 February 2002
DOI:https://doi.org/10.1103/PhysRevB.65.214422
©2002 American Physical Society