High-field ESR spectroscopy of the spin dynamics in La1xSrxMnO3 (x<~0.175)

D. Ivannikov, M. Biberacher, H.-A. Krug von Nidda, A. Pimenov, A. Loidl, A. A. Mukhin, and A. M. Balbashov
Phys. Rev. B 65, 214422 – Published 4 June 2002
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Abstract

High-field electron-spin-resonance (ESR) experiments have been carried out in single crystals of La1xSrxMnO3 in the concentration range 0<~x<~0.175. Different quasioptical arrangements have been utilized for frequencies 40<~ν<~700GHz and for magnetic fields B<~12T. A splitting of the antiferromagnetic resonance (AFMR) mode is observed in the magnetic field for the parent compound LaMnO3, in agreement with the antiferromagnetic structure of this material. Abrupt changes in the AFMR frequencies have been observed around x0.025, and were attributed to a transition between a pure antiferromagnetic and a canted state. For increasing Sr doping the observed AFMR modes are split even in a zero field, which can be naturally explained using a concept of a canted magnetic structure for x<0.1. In La0.825Sr0.175MnO3 the ESR spectra are consistent with the ferromagnetic and metallic state. The lines of ferromagnetic resonance and ferromagnetic antiresonance can be clearly observed. For intermediate concentrations 0.1<~x<~0.15 complicated ESR spectra were observed, which can be well explained by a single ferromagnetic resonance mode and taking electrodynamic effects into account.

  • Received 1 February 2002

DOI:https://doi.org/10.1103/PhysRevB.65.214422

©2002 American Physical Society

Authors & Affiliations

D. Ivannikov, M. Biberacher, H.-A. Krug von Nidda, A. Pimenov*, and A. Loidl

  • Experimentalphysik V, Elektronische Korrelationen und Magnetismus, Institut für Physik, Universität Augsburg, 86135 Augsburg, Germany

A. A. Mukhin

  • General Physics Institute of the Russian Academy of Sciences, 119991 Moscow, Russia

A. M. Balbashov

  • Moscow Power Engineering Institute, 105835 Moscow, Russia

  • *Corresponding author. Email address: Andrei.Pimenov@Physik.Uni-Augsburg.DE

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Vol. 65, Iss. 21 — 1 June 2002

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