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Enhancement of the magnetoresistance at the Curie temperature of the ferromagnetic insulator La1.5Sr0.5MnRhO6

A. I. Coldea, I. M. Marshall, S. J. Blundell, J. Singleton, L. D. Noailles, P. D. Battle, and M. J. Rosseinsky
Phys. Rev. B 62, R6077(R) – Published 1 September 2000
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Abstract

We report a study of the magnetic and electrical properties of the ferromagnetic insulator La1.5Sr0.5RhMnO6. A significant magnetoresistance is found in this system which is largest at the Curie temperature (TC) even though there is no metal-insulator transition. The electrical transport is found to be activated above TC and described by a variable range hopping law below TC. Above TC the carriers are magnetic polarons with a size which increases as the temperature approaches the magnetic transition. Rh substitution preserves ferromagnetic ordering, in contrast with the effect of other dopants on the B sites, but modifies the electrostatic potential leading to carrier localization. We attribute the peak in the magnetoresistance at TC to the field-induced suppression of critical spin fluctuations which modulate the energetic barriers seen by the carriers.

  • Received 8 May 2000

DOI:https://doi.org/10.1103/PhysRevB.62.R6077

©2000 American Physical Society

Authors & Affiliations

A. I. Coldea, I. M. Marshall, S. J. Blundell, and J. Singleton

  • Clarendon Laboratory, University of Oxford, Parks Road, Oxford OX1 3PU, United Kingdom

L. D. Noailles*, P. D. Battle, and M. J. Rosseinsky*

  • Inorganic Chemistry Laboratory, University of Oxford, South Parks Road, Oxford OX1 3QR, United Kingdom

  • *Present address: Department of Chemistry, University of Liverpool, Liverpool L69 7ZD, UK.

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Vol. 62, Iss. 10 — 1 September 2000

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