Temperature and doping-level dependence of magnetic order in La2xSrxNiO4+δ studied by muon spin rotation

Th. Jestädt, K. H. Chow, S. J. Blundell, W. Hayes, F. L. Pratt, B. W. Lovett, M. A. Green, J. E. Millburn, and M. J. Rosseinsky
Phys. Rev. B 59, 3775 – Published 1 February 1999
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Abstract

We report muon-spin-rotation (μSR) measurements on a series of compounds with composition La2xSrxNiO4+δ with strontium doping level x between 0 and 1. A magnetic transition is found in all the samples studied, which occurs at a composition-dependent temperature, TM. Below TM clear precession signals are observed in zero applied magnetic field for all x, indicating the existence of at least short-range magnetic order on a time scale longer than 108 s. Above TM the magnetic correlation times decrease by several orders of magnitude. At x0.33, we find peaks in both TM and the zero-temperature staggered magnetization, an observation which we attribute to the higher degree of localization of the holes at this doping level. The measurements of TM as a function of x extend the determination of Néel temperatures by previous neutron diffraction and μSR measurements.

  • Received 29 June 1998

DOI:https://doi.org/10.1103/PhysRevB.59.3775

©1999 American Physical Society

Authors & Affiliations

Th. Jestädt*, K. H. Chow, S. J. Blundell, W. Hayes, F. L. Pratt, and B. W. Lovett

  • Clarendon Laboratory, University of Oxford, Parks Road, Oxford, OX1 3PU, United Kingdom

M. A. Green, J. E. Millburn, and M. J. Rosseinsky

  • Inorganic Chemistry Laboratory, University of Oxford, South Parks Road, Oxford, OX1 3QR, United Kingdom

  • *Electronic address: t.jestadt@physics.ox.ac.uk
  • Present address: Department of Physics, Lehigh University, 16 Memorial Drive East, Bethlehem, PA 18015.

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Vol. 59, Iss. 5 — 1 February 1999

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