Pt195 spin dynamics and Knight shift in single crystals of UPt3

Moohee Lee, G. F. Moores, Y.-Q. Song, W. P. Halperin, W. W. Kim, and G. R. Stewart
Phys. Rev. B 48, 7392 – Published 1 September 1993
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Abstract

Pt195 nuclear-magnetic-resonance measurements were performed on aligned single-crystal whiskers of UPt3 for temperatures from 4 to 50 K. A special alignment technique allows us to produce samples with very good c-axis alignment and to work with the field parallel to the c axis with an excellent signal-to-noise ratio. Combining the Knight shift and spin-lattice-relaxation data, we show a continuous crossover from paramagnetic behavior above 40 K toward a degenerate-Fermi-liquid behavior below 5 K. Antiferromagnetic spin fluctuations appear to be responsible for this crossover process, and dominate all low-frequency magnetic properties of this compound. The anisotropy ratios of both the spin-lattice and the spin-spin relaxation rates are found to be temperature independent. Analyzing these ratios we find that the imaginary part of the dynamic spin susceptibility is slightly stronger in the basal plane.

  • Received 29 March 1993

DOI:https://doi.org/10.1103/PhysRevB.48.7392

©1993 American Physical Society

Authors & Affiliations

Moohee Lee, G. F. Moores, Y.-Q. Song, and W. P. Halperin

  • Department of Physics and Astronomy and Materials Research Center, Northwestern University, Evanston, Illinois 60208

W. W. Kim and G. R. Stewart

  • Department of Physics, University of Florida, Gainesville, Florida 32611

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Vol. 48, Iss. 10 — 1 September 1993

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