Abstract
Stage-2 graphite intercalation compounds behave magnetically like a quasi-two-dimensional Heisenberg ferromagnet with XY spin anisotropy. The spin symmetry continuously changes from Heisenberg-like at c=0 to XY-like at c=1. The effect of spin anisotropy on the critical behavior of these compounds has been studied by using ac and dc magnetic susceptibility. The ratio of critical temperature to Curie-Weiss temperature FTHETA as a function of effective XY spin anisotropy parameter is well described by /FTHETA=+B with A=0.229, B=0.224, and the crossover exponent φ(=1.34). The first and second terms of /FTHETA are due to the spin anisotropy effect in the two-dimensional system and the three-dimensional effect, respectively. The extrapolated value of at =1 may give an estimate for the ratio of the Kosterlitz-Thouless temperature to the intraplanar exchange interaction.
- Received 27 March 1992
DOI:https://doi.org/10.1103/PhysRevB.46.5311
©1992 American Physical Society