Abstract
Temperature-dependent, low-field (50 Oe) dc magnetic susceptibility (χ) studies are reported for the randomly diluted fcc system O. The studies, using powder samples, covered the temperature range 1.6–300 K and the composition range 0.10≤p<1. Variations of the Néel temperature , the Curie-Weiss temperature Θ, the Curie constant C, the low-temperature magnetization M, and the lattice constant with p are reported. The observed percolation threshold =0.13 agrees well with the predicted value of =0.136 for fcc system with nearest-neighbor and next-nearest-neighbor interactions included. The variation of Θ(p) and (p) with p is found to be linear whereas that of t=(p)/(1) is more complex, showing a crossover near p=0.45, where t/ changes sign. Calculations are needed to explain this observed t versus p variation. For
χ below depends upon how the sample is cooled through , and the hysteresis and time dependence (relaxation) of χ are observed at 4.2 K if the sample is cycled through a higher field (6 kOe). These observations are not fully understood. An estimate of the exchange constants for the O system is given.
- Received 1 December 1986
DOI:https://doi.org/10.1103/PhysRevB.35.6847
©1987 American Physical Society